Copper nanoparticles supported on zinc oxide as efficient catalyst for the N-Arylation of (Hetero)cyclic and acyclic amides

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dc.catalogadorpva
dc.contributor.authorMoglie, Yanina
dc.contributor.authorMascaro, Evangelina
dc.contributor.authorZacconi, Flavia C. M.
dc.contributor.authorRadivoy, Gabriel
dc.date.accessioned2023-08-23T20:25:08Z
dc.date.available2023-08-23T20:25:08Z
dc.date.issued2021
dc.description.abstractCopper nanoparticles (CuNPs) supported on ZnO are highly active and selective heterogeneous catalyst for the N-arylation of cyclic and acyclic amides (Golberg coupling). The reaction conditions are mild, featuring K3PO4 as a base and N,N'-dimethylethylendiamine (DMEDA) as ligand in refluxing acetonitrile. The CuNPs/ZnO catalyst can be recovered and reused in six cycles with only little loss of activity. The methodology can be successfully scaled up to gram scale without decreasing the catalytic activity.
dc.description.funderArgentinian Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET)
dc.description.funderAgencia Nacional de Promocion Cientifica y Tecnologica (ANPCyT, Prest. BID)
dc.description.funderUniversidad Nacional del Sur (UNS, Argentiina)
dc.description.funderANID/CONICYT FONDECYT (Chile)
dc.fechaingreso.objetodigital2023-08-23
dc.format.extent6 páginas
dc.fuente.origenWOS
dc.identifier.doi10.1002/slct.202101011
dc.identifier.eissn2365-6549
dc.identifier.urihttps://doi.org/10.1002/slct.202101011
dc.identifier.urihttps://repositorio.uc.cl/handle/11534/74479
dc.identifier.wosidWOS:000656953000001
dc.information.autorucEscuela de Química; Zacconi, Flavia C. M.; 0000-0002-3676-0453; 1011127
dc.issue.numero18
dc.language.isoen
dc.nota.accesoContenido parcial
dc.pagina.final4417
dc.pagina.inicio4412
dc.publisherWILEY-V C H VERLAG GMBH
dc.revistaChemistrySelectes_ES
dc.rightsacceso restringido
dc.subjectLactamses_ES
dc.subjectAmideses_ES
dc.subjectN-arylationes_ES
dc.subjectCopper nanoparticleses_ES
dc.subjectHeterogeneous catalystes_ES
dc.subjectCoupling reactions scopees_ES
dc.subjectAryl halideses_ES
dc.subjectC-Nes_ES
dc.subjectGoldberg reactiones_ES
dc.subjectAmidationes_ES
dc.subjectComplexeses_ES
dc.subjectAminationes_ES
dc.subjectMildes_ES
dc.subjectHeterocycleses_ES
dc.subjectBromideses_ES
dc.subject.ddc510
dc.subject.deweyMatemática física y químicaes_ES
dc.titleCopper nanoparticles supported on zinc oxide as efficient catalyst for the N-Arylation of (Hetero)cyclic and acyclic amides
dc.typeartículo
dc.volumen6
sipa.codpersvinculados1011127
sipa.indexWoS
sipa.trazabilidadWOS;18-03-2022
sipa.trazabilidadORCID;2023-08-21
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